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Sempill or Semple may refer to:
- Francis Sempill (1616?–1682), Scottish writer, son of Robert the younger
- James Sempill (1566–1626), Scottish courtier and diplomat
- Hugh Sempill (1596–1654), Scottish mathematician
- Robert Sempill (c.1530–1595), Scottish balladeer
- Robert Sempill the younger (1595?–1663?), Scottish writer, son of Robert
- William Forbes-Sempill, 19th Lord Sempill (1893–1965), Scottish pioneering aviator and Japanese spy.